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Detector and Measurement Interests for n_TOF EAR2

Detector and Measurement Interests for n_TOF EAR2. J. Billowes, C. Guerrero, D. Jenkins, M. Vermeulen , T. Ware, T. Wright. Motivating Measurement: 13 C(n,  ) 14 C.

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Detector and Measurement Interests for n_TOF EAR2

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  1. Detector and Measurement Interests for n_TOF EAR2 J. Billowes, C. Guerrero, D. Jenkins, M. Vermeulen, T. Ware, T. Wright

  2. Motivating Measurement: 13C(n,)14C • Reaction is of great UK interest due to large volume of reactor graphite (130,000 tonnes) from earlier Magnox reactors.14C is a major activation product requiring consideration in decommissioning • Contribution from 13C(n,)14C is source of uncertainty due to low cross section, based on theory • Major issue with measurement is very low capture / scattering ratio (order of 10-3) • High quality sample and new measurement/analysis techniques needed

  3. 13C(n,)14C Other libraries; EAF-2007, EAF-2010, RUSFOND-2010 = JEFF-3.0/A

  4. Contributions to New Detector Arrays • Manchester/York are assembling a EPSRC nuclear data proposal to include detector characterisation work • York have submitted proposal to UK NDA (nuclear decommissioning authority) for studentship to investigate 13C(n,)14C measurement, including detector characterisation • Manchester have facilities and expertise for design and construction of detector assemblies (e.g. TAC array) • York are heavily involved in the PARIS collaboration – which aims to build a calorimeter for SPIRAL2 using lanthanum bromide • York also involved in the NuPNET scheme, GANAS which is characterising novel scintillators and photosensors

  5. Possible detection techniques for 13C(n,g) • Exploit the high gamma-ray sum energy (~ 8 MeV) released from 13C(n,g) in order to discriminate the capture channel • Use novel scintillators like LaBr3or CeBr3. No need for 4πsolid angle but need absolute detector efficiency (from simulations) • Could combine with a C6D6 measurement (for cross section), using the spectroscopy measurement to gain reaction selectivity (no clear idea how to combine the two methods) • Investigate scintillators with high energy resolution and neutron-gamma discrimination e.g. CLYC from Hilger Crystals/RMD • Pair spectrometer – i.e. detect positron/electron pairs from the high energy capture events

  6. Testing with 13C(n,)14C ‘Surrogate’ • 12C(n,)13C cross section is similar to 13C(n,)14C • Could use existing 12C background measurements to test discrimination techniques

  7. Detection Techniques • Discriminate on deposited energy in TAC?

  8. Lanthanum bromide • Very high energy resolution – 3% at 662-keV • York is member of PARIS • PARIS has 28 phoswich detectors (2” cubic LaBr3 + CsI) • Intention is to build full calorimeter of 200

  9. Other new materials might be of interest for neutron-gamma discrimination e.g. CLYC

  10. Pair spectrometer • Pair spectrometers can measure positron-electron pairs from internal pair transitions e.g. 8 MeV transition in 14C following capture • A low probability process (10-3 per decay) • But, in principle, 100% clean as pairs can be moved away from the target avoiding neutron scattering effect • What is plausible efficiency though? – could be less than a % which would make it a very selective but very low overall efficiency technique • Needs modelling

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