Entropy favors asymmetry in colloidal self assembly
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Entropy Favors Asymmetry in Colloidal Self-Assembly. Guangnan Meng, Natalie Arkus, Michael P. Brenner, and Vinothan N. Manoharan.

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Entropy Favors Asymmetry in Colloidal Self-Assembly

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Entropy favors asymmetry in colloidal self assembly

Entropy Favors Asymmetry in Colloidal Self-Assembly

Guangnan Meng, Natalie Arkus, Michael P. Brenner, and

Vinothan N. Manoharan

Two self-assembled colloidal clusters, as seen under the optical microscope. The cluster on the left, a tri-tetrahedron, and the cluster on the right, an octahedron, have the same energy. But in an experiment where both clusters are allowed to form randomly in solution, the less symmetric tri-tetrahedron occurs more than twenty times as often as the highly symmetric octahedron because of the many more ways to form the tri-tetrahedron. The findings illustrate, in a tangible way, what entropy is and how it determines the structures of small self-assembled materials.

Harvard MRSECDMR-0820484 D.A. Weitz and C.M. Friend


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