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Whitecaps, sea-salt aerosols, and climate

Physical Oceanography Dissertation Symposium. Whitecaps, sea-salt aerosols, and climate. Magdalena D. Anguelova. College of Marine Studies, University of Delaware. June 17-21, 2002 Breckenridge, Colorado. Outline. Background. Why?. How?. Work. Results.

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Whitecaps, sea-salt aerosols, and climate

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  1. Physical Oceanography Dissertation Symposium Whitecaps, sea-salt aerosols, and climate Magdalena D. Anguelova College of Marine Studies, University of Delaware June 17-21, 2002 Breckenridge, Colorado

  2. Outline • Background Why? How? • Work • Results What?

  3. Aerosol effects IPCC, 2001

  4. Aerosol radiative forcing • Defined as… • Assessment: Effect of anthropogenic aerosols = • Effect of all aerosols – Effect of natural aerosols natural

  5. Natural aerosols; Baseline of an unperturbed atmosphere. Background atmosphere

  6. Background baseline • Natural aerosols; • Baseline of an unperturbed atmosphere. Sea-salt aerosols Sea-salt aerosols are the dominant aerosol species in background atmosphere.

  7. Formation of sea-salt aerosols • Sea spray; • Droplet sizes: • 0.5-500 m; • < 20 m; • Sea-salt aerosols: • Phase state; • Sizes: 0.025 to 20 m.

  8. Motivation Sea-salt aerosol effects must be accounted for in climate models.

  9. Modeling sea-salt aerosols Generation • Generation; • Transport; • Diffusion and convection; • Chemical and physical transformations: • in clear air; • in clouds; • below clouds; • Wet and dry deposition.

  10. (Monahan and O’Muircheartaigh, 1980) Explicit forms for 4 size regions covering 1.6 to 500 m range. Andreas (2001) Sea spray generation function Rate of production of sea spray per unit area per increment of droplet radius, r (s-1 m-2m-1). Best

  11. r0 1.6 m Measurements (Monahan and O’Muircheartaigh, 1986) W(U10, T, Ts , S, f , d , C) ) ,Ts ,f ,C) ,S ,d Improved generation function? 0.1 , Ts , f , C) , T , S , d Whitecap coverage

  12. Need for a database W (U10 , T, Ts , S, f , d , C) 10 2 16 11 15 12 4 13 7 6 5 1 3 9 14

  13. 307 points 477 points Need of a database W (U10 , T, Ts , S, f , d , C) New method 10 2 16 11 15 12 4 13 7 6 5 1 3 9 14

  14. Outline • Background • Work • Results

  15. Emissivity of foam-free ocean is low. e – es – er W = ef – es – er Method concept e  as W  • Emissivity of foam-covered ocean is high. • Ocean emissivity is composite e = (es + er)(1-W ) + W ef

  16. TB, V, L SSM/I Radiative transfer equation AVHRR NOAA Ts, S Fresnel formula, Debye equation Ts, S Fresnel formula, empirical relation SSM/I AVHRR U10, Ts Empirical relation The task: calculate emissivities • Composite emissivity e: • Specular emissivity es: • Foam emissivity ef : • Roughness correction Der:

  17. Valid estimation of W e < es + er W < 0 2 – 10 %

  18. Error of W

  19. Method accuracy Count Relative error, W/W (%)

  20. Whitecap coverage 27 March 1998

  21. Validation with in situ data

  22. Validation with in situ data • Magnitude; • Trend: • Suppression at high winds; • Enhancement at moderate winds. • Variability!

  23. Outline • Background • Work • Results

  24. Database • Content: • Daily and monthly estimates of W and W for the entire 1998; • Collocated measurements of U10, Ts, S; Use: • Investigate spatial and temporal characteristics of global whitecap coverage; • Evaluate whitecap contribution to climate processes. • Parameterize effects of additional factors on whitecaps;

  25. Same magnitude; Different spatial features: More uniform; 3% instead of 1%. • W U103 Spatial distribution March 1998

  26. Wind speed,U10 (m s-1) Sea surface temperature,Ts(oC) Effects of additional factors March 1998 • Wind fetch and duration; • Surface-active material.

  27. Natural climate agent; Average: 0.11 W m-2; Ocean surface albedo • Anthropogenic agents: • Stratospheric ozone (0.18 W m-2) • Biomass burning (0.21 W m-2) • Land use (0.22 W m-2) Radiative flux changes, F (W m‑2)

  28. 5 – 150 cm h-1; Average: 56.8 cm h-1; Tropics are source of CO2; Southern Ocean is sink of CO2. CO2 transfer velocity Flux = kCO2C CO2 transfer velocity, kCO2 (cm h‑2)

  29. Improved generation function? r0 1.6 m 0.1 Measurements (Monahan and O’Muircheartaigh, 1986) W(U10, T, Ts , S, f , d , C) W(U10)

  30. Modified generation function   m Andreas, 2001   m Monahan et al., 1986   m Future work Assimilating new method estimates

  31. Ts in places with U10 = 10 m s-1 Ts in places with U10 = 15 m s-1 Sea surface temperature, TsoC Sea-salt aerosol loading • Magnitude; • Weak wind dependence;

  32. Haywood et al., 1999 Model - Experiment Spatial distribution of sea-salt 1105410571051106 Number flux, dF/dr0 (# m-1 m-2 s-1) Direct effect: 15 W m-2

  33. Conclusions • Whitecap coverage estimation • Whitecap coverage database • Generation of sea-salt aerosols

  34. ????? ?????

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