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Au-shell cavity mode - Mie calculations

Au-shell cavity mode - Mie calculations. R core = 228 nm R total = 266 nm t Au = 38 nm medium = silica. cavity mode 700 nm. cavity mode 880 nm. 880 nm = 340 THz. 1. Finite Difference Time Domain method. k y. E x. Step 1: Excitation. Step 2: Relaxation. Step 3: Fourier Transform.

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Au-shell cavity mode - Mie calculations

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  1. Au-shell cavity mode - Mie calculations Rcore = 228 nm Rtotal = 266 nm tAu = 38 nm medium = silica cavity mode 700 nm cavity mode 880 nm 880 nm = 340 THz 1

  2. Finite Difference Time Domain method ky Ex Step 1: Excitation Step 2: Relaxation Step 3: Fourier Transform Plane wave excitation on and off resonance stores some energy in particle Fast Fourier transform of the relaxation E(t) to generate frequency spectrum Particle oscillates, reemitting at its resonance frequency 2

  3. Snapshots- Au shell (R=266 nm, tAu = 38 nm) in silica box (1.5x1.5 μm2) +2 +1 Ex 0 -1 -2 excitation off-resonance at 150 THz (2 μm) E-field monitor in center 335 THz (895 nm) Fast Fourier Transform p=1.3x1016 rad/s =1.25 x1014 rad/s d=9.54 3

  4. Snapshots- Au shell (R=266 nm, tAu = 38 nm) in silica box (1.5x1.5 μm2) +2 +1 Electric field intensity max= 6.5 at center 5 Ex 0 cavity mode! -1 0 excitation on-resonance at 335 THz (895 nm) -2 excitation off-resonance at 150 THz (2 μm) 4

  5. Cavity parameters • Quality factor Q=35 • The maximum field enhancement within the core amounts to a factor of 6.5 • The mode volume V=0.2 (/n)3 … 102-103 smaller thanthan that in micordisc/microtoroid WGM cavities • A characteristic Purcell factor – assuming homogeneous field distribution in the cavity core and =895 nm

  6. Cavity optimization A characteristic Purcell factor assuming homogeneous field distribution in the cavity core, =895 nm and Q=150:

  7. Cavity mode is tunable - T-matrix vs FDTD calculations Penninkhof et al, JAP 103, 123105 (2008) 7

  8. Cavity mode is tunable by shape -oblate Au shell spheroid T / 240 THz L / 410 THz aspect ratio=2.5 8

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