Phenomenological properties of nuclei. 1) Introduction - nucleon structure of nucleus 2) Sizes of nuclei 3) Masses and bounding energies of nuclei 4) Energy states of nuclei 5) Spins. 6) Magnetic and electric moments 7) Stability and instability of nuclei 8) Exotic nuclei
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Phenomenological properties of nuclei
1) Introduction - nucleon structure of nucleus
2) Sizes of nuclei
3) Masses and bounding energies of nuclei
4) Energy states of nuclei
6) Magnetic and electric moments
7) Stability and instability of nuclei
8) Exotic nuclei
9) Nature of nuclear forces
Introduction – nucleon structure of nuclei.
Atomic nucleus consists of nucleons (protons and neutrons).
Number of protons (atomic number) – Z.
Total number nucleons (nucleon number) – A.
Number of neutrons – N = A-Z.
Different nuclei with the same number of protons – isotopes.
Different nuclei – nuclides.
Different nuclei with the same number of neutrons – isotones.
Nuclei with N1 = Z2 and N2 = Z1 – mirror nuclei
Different nuclei with the same number of nucleons – isobars.
Neutral atoms have the same number of electrons inside atomic electron shell as protons inside
Proton number gives also charge of nucleus: Qj = Z·e
(Direct confirmation of charge value in scattering experiments – from Rutherford equation
for scattering (dσ/dΩ)= f(Z2))
Atomic nucleus can be relatively stable in ground state or in excited state to higher
energy – isomers (τ > 10-9s).
Stable nuclei have A and Z which fulfill approximately empirical equation:
Reliably known nuclei are up to Z=112 in present time (discovery of nuclei with Z=114, 116 (Dubna) needs confirmation).
Nuclei up to Z=83 (Bi) have at least one stable isotope. Po (Z=84) has not stable isotope.
Th , U a Pu have T1/2comparable with age of Earth.
Maximal number of stable isotopes is for Sn (Z=50) - 10 (A =112, 114, 115, 116, 117, 118, 119, 120,
Total number of known isotopes of one element is till 38.
Number of known nuclides: > 2800.
Sizes of nuclei
Distribution of massorchargein nucleus are determined.
We use mainly scattering of charged or neutral particles on nuclei.
Density ρ of matter and charge is constant inside nucleus and we observe fast density decrease on the nucleus boundary. The density distribution can be described very well for spherical nuclei by relation (Woods-Saxon):
where α is diffusion coefficient. Nucleus radius R is distance from the center, where density is half of maximal value. Approximate relation R = f(A)can be derived from measurements:
R = r0A1/3
where we obtained from measurementr0 = 1,2(1) 10-15 m = 1,2(2) fm (α = 1,8 fm-1).This shows on permanency of nuclear density. Using Avogardo constant
we obtain 1017 kg/m3.
or using proton mass:
High energy electron scattering (charge distribution) smaller r0.
Neutron scattering (mass distribution) larger r0.
Larger volume of neutron matter is done by larger number
of neutrons at nuclei (in the other case the volume of protons
should be larger because Coulomb repulsion).
Neutrons:mnc2 >> EKIN → → EKIN > 20 MeV
Deformed nuclei– all nuclei are not spherical, together with smaller values of deformation of some nuclei in ground state the superdeformation(2:1 3:1) was observed for highly excited states. They are determined by measurements of electric quadruple moments and electromagnetic transitions between excited states of nuclei.
Neutron and proton halo– light nuclei with relatively large excess of neutrons or protons
→ weakly bounded neutrons and protons form halo around central part of nucleus.
Experimental determination of nuclei sizes:
1) Scattering of different particles on nuclei:Sufficient energy of incident particles is necessary for studies of sizesr = 10-15m. De Broglie wave lengthλ = h/p < r:
Electrons: mec2 << EKIN → λ = hc/EKIN → EKIN > 200 MeV
2) Measurement of roentgen spectra of mion atoms:They have mions in place of electrons (mμ = 207 me):μ,e – interact with nucleus only by electromagnetic interaction. Mions are ~200 nearer to nucleus → „feel“ size of nucleus(K-shell radius is for mion at Pb 3 fm ~ size of nucleus)
3) Isotopic shift of spectral lines:The splitting of spectral lines is observed in hyperfine structure of spectra of atoms with different isotopes – depends on charge distribution – nuclear radius.
4) Coulomb energy of nucleus: Reduction of Coulomb energy ECand the same reduction off binding energy of nucleus (energy of uniformly charged sphere)
Mirror nuclei – same nuclear binding energy, different Coulomb energy. Difference of binding energy is given by EC difference.
5) Study of α decay:The nuclear radius can be determined using relation between probability of α particle production and its kinetic energy.
Masses of nuclei
Nucleus hasZprotons andN=A-Zneutrons. Naive conception of nuclear masses:
M(A,Z) = Zmp+(A-Z)mn
wherempis proton mass(mp 938.27 MeV/c2) andmnis neutron mass (mn 939.56 MeV/c2)
whereMeV/c2 = 1.78210-30 kg, we use also mass unit:mu = u= 931.49 MeV/c2 = 1.66010-27 kg. Then mass of nucleus is given by relative atomic massAr=M(A,Z)/mu.
Real masses are smaller – nucleus is stable against decay because of energy conservation law.
Mass defect ΔM:
ΔM(A,Z) = M(A,Z) – (Zmp + (A-Z)mn)
It is equivalent to energy released by connection of single nucleons to nucleus -binding energy B(A,Z) = - ΔM(A,Z) c2
Binding energy per one nucleonB/A:
Maximal is for nucleus56Fe (Z=26, B/A=8.79 MeV).
Possible energy sources:
8.79 MeV/nucleon 1.4·10-13 J/1,66·10-27 kg = 8.7·1013 J/kg
Binding energy per one nucleon for stable nuclei
(gasoline burning: 4.7·107 J/kg)
forisFB = QvB
Measurement of masses and binding energies:
Mass spectrographsandspectrometersuse particle motion in electric and magnetic fields:
Massm=p2/2EKINcan be determined by comparison of momentum and kinetic energy. We use passage of ions with chargeQthrough“energy filter” and “momentum filter”, which are realized using electric and magnetic fields:
and thenF = QE
The study of Audi and Wapstra from 1993 (systematic review of nuclear masses) names 2650 different isotopes. Mass is determined for 1825 of them.
Frequency of revolution in magnetic fieldof ion storage ring is used. Momenta are equilibrated byelectron cooling → for different masses → different velocity and frequency.
Comparison of frequencies (masses)
of ground and isomer states of
52Mn. Measured at GSI Darmstadt
Electron cooling of
storage ring ESR at GSI Darmstadt
1) We measure energy of γ quantum essential for deuteron split:
AtGSI Darmstadtfragment separator(FSR) makes possible to produce different isotopes andstorage ring(ESR) makes possible to measure big number of nuclear masses. Accuracy isΔM = 0,1 MeV/c2, that means relative accuracyΔM/M ~ 10-6. Possibility to measure also very short isotopes τ > 30 s (with electron cooling), τ ≈ μs (without electron cooling).
Similar device is atCERN (ISOLDE)
Exploitation of reaction energy balance:
Useful also in the case where mass spectroscopy is not working (neutral particles).
Determination of neutron mass as example:
2) Deuteron mass is:md = mn + mH - B
3) Masses of hydrogen and deuteron are measured by spectroscopy.
4) Neutron mass is:mn = (md - mH) + B.
Masses of other instable particles and nuclei can be determined by this method (ΔM/M ~ 10-8).
Are nucleons localized at nuclei?B/A 8 MeV /AEnergy necessary for nucleon separation 8 MeV
De Broglie wave length = h/p binding state condition2r = n(nnatural number) /2
shows typical size.8 MeV << 939 MeV→ nonrelativistic approximation
Agree with nuclear sizes.
Can be electrons localized at nuclei?Electron with EKIN=8 MeV is relativistic even ultrarelativistic:
Excited energy states
Nucleus can be both in ground state and in state with higher energy –excited state
Every excited state – corresponding energy→ energy level
Quantum physics → discrete values of possible energies
Scheme of energy levels:
Deexcitation of excited nucleus from higher level to lower one byphoton irradiation (gamma ray)or direct transfer of energy to electron from electron cloud of atom –irradiation of conversion electron. Nucleus is not changed. Or by decay (particle emission). Nucleus is changed.
Energy level structure of 66Cu nucleus (measured at GANIL – France, experiment E243)
Obtaining of excited state of nuclei:
The big number of different isotopes can be produced using the fragment separators and radioactive beams make possible.
obtained by device
Measurement of properties of transitions between excited states:
1) Energy spectra and angular distribution of gamma rays
2) Energy spectra of conversion electrons
Measurement of excited state properties:
Energy spectra and angular distribution of particles
from scattering or reactions
Gamma ray spectrum of deexcitation of 70Ni levels (experiment E243)
Classically angular momentum is define as . At quantum physic by appropriate operator,
which fulfill commutating relations:
1) Eigenvalues are , where number I = 0, 1/2, 1, 3/2, 2, 5/2 … angular momentum magnitude is |I| = ħ [I(I+1)]1/2
2) From commutation relations it results, that vector components can not be observed individually.
Simultaneously and only one component – for example Iz can be observed.
5) Superposition for single nucleon leads to j = l 1/2.Superposition for system of more
particles is diverse.Extreme cases:
Spins of nuclei
Protons and neutrons have spin 1/2. Vector sum of spins and orbital angular momenta is
total angular momentum of nucleus I which is named as spin of nucleus
Orbital angular momenta of nucleons have integral values → nuclei with even A – integral spin
nuclei with odd A – half-integral spin
There are valid such rules:
3) Components (spin projections) can take values Iz = Iħ, (I-1)ħ, (I-2)ħ, … -(I-1)ħ, -Iħ together 2I+1
4) Angular momentum is given by number I = max(Iz). Spin corresponding to orbital angular
momentum of nucleons is only integral: I ≡ l = 0, 1, 2, 3, 4, 5, … (s, p, d, f, g, h, …),
intrinsic spin of nucleon is I ≡ s = 1/2.
Electric quadruple momentQ: gives difference of charge distribution from spherical. Assumption:
Nucleus is rotational ellipsoid with uniformly distributed chargeZe:
(c,aare main split axles of ellipsoid) deformationδ = (c-a)/R = ΔR/R
Magnetic and electric momenta
Magnetic dipole momentμ is connected to existence of spin I and charge Ze. It is given by relation:
where g is g-factor(sometimes named also as
gyromagnetic ratio) and μj is nuclear magneton:
For point like particle g = 2 (for electron agreement μe = 1.0011596 μB). For nucleons μp = 2.79 μj and μn = -1.91 μj – anomalous magnetic moments show complicated structure of these particles.
Magnetic moments of nuclei are only μ = -3 μj 10 μj, even-even nucleiμ = I = 0 → confirmation
of small spins, strong pairing and absence of electrons at nuclei.
Electric dipole momentum: is connected with charge polarization of system. Assumption: nuclear charge in the ground state is distributed uniformly → electric dipole momentum is zero.
Agree with experiment.
Magnetic dipole moments of nucleus are measured by their interaction with magnetic field. Energy of magnetic dipolein magnetic field is:
Results of measurements:
1) Most of nuclei have Q = 10-2910-30 m2 → δ ≤ 0.1
2) In the region A ~ 150 180 and A ≥ 250 large values are measured:Q ~ 10-27 m2. They are larger than nucleus area. → δ ~ 0.2 0.3 → deformed nuclei.
Generally apply to:
1) All odd electric multiple moments disappeared
2) All even magnetic multiple moments disappeared
3) For state with total angular momentum I, mean value of all moments, which order of multiple L > 2I disappeared. Nuclei with I = 0,1/2 has not electric quadruple moment.
Measurement of magnetic moments
A) Magnetic moments of nuclei can be obtained from splitting hyperfine structure (interaction
between electron cloud and nucleus).
B)On the base of motion of magnetic dipole through magnetic fields:
C) Measurement of magnetic resonance: Sample is placed to homogeneous magnetic field. Energy
difference corresponding to different projections of angular momentum IZ : ΔEmag = gμΔIZB.
For dipole transitions ΔIZ = ±1 : ΔEmag = ħ L = gμB → L = (1/ħ) gμB where Lis
Larmor frequency. Resonance is observed by energy absorption at induction coil.
Stability and instability of nuclei
Stable nuclei: for small A (<40) is valid Z = N, for heavier nuclei N 1,7 Z. This dependence can be express more accurately by empirical relation:
For stable heavy nuclei excess of neutrons → charge density and destabilizing influence of Coulomb
repulsion is smaller for larger number of neutrons.
N Z number of stable nuclei
even even 156
even odd 48
odd even 50
odd odd 5
Even-even nuclei are more stable→ existence of pairing
Magic numbers – observed values of N and Z with increased stability.
At 1896 H. Becquerel observed first sign of instability of nuclei – radioactivity. Instable
Alpha decay → nucleus transformation by 4He irradiation
Beta decay → nucleus transformation by e-, e+ irradiation or capture of electron from atomic cloud
Gamma decay → nucleus is not changed, only deexcitation by photon or converse electron irradiation
Spontaneous fission → fission of very heavy nuclei to two nuclei
Proton emission → nucleus transformation by proton emission
Nuclei with livetime in the ns region are studied in present time. They are bordered by:
proton stability border during leave from stability curve to proton excess (separative energy
of proton decreases to 0)and neutron stability border – the same for neutrons.Energy level
width Γ of excited nuclear state and its decay time τ are connected together by relation τΓ ≈ h. Boundery for decay time Γ < ΔE (ΔE – distance of levels) ΔE~ 1 MeV→ τ >> 6·10-22s.
Nuclei far away from stability curve:
1) with large excess of neutrons
2) with large deficit of neutrons (excess of protons)
Effort to study all isotopes between boundaries of proton and neutron stability.
Double magic nuclei: 100Sn is such nucleus with maximal numbers of neutrons and protons
Firstly observed at GSI Darmstadt at Germany and at GANIL Caen at France
Highly excited states:
1) with very high energy
2) with very high spin
3) with large deformation → quadruple moments
(superdeformed till hyperdeformed)
Cases of observation of nucleus
100Sn at GSI Darmstadt
Device for exotic nuclei studies at GSI Darmstadt
Superheavy nuclei:for large A and Z stability is increasing – existence of magic numbers → existence of stability island. Nuclei up to Z = 112 (mainly GSI Darmstadt, JINR Dubna a Berkeley) were confirmed, Discovery of nuclei with Z = 114 (Dubna) a Z = 116 a 118 (Berkeley) need confirmation.
Table of isotopes in the region of superheavy elements (situation in 2000)
Hypernuclei: One or more neutrons are changed by neutral hyperon Λ. ΛH3, ΛHe5, ΛLi9,
ΛO16, ΛFe56, ΛBi209, ΛΛHe6, ΛΛBe8). Other hyperons (Σ, Ξ, Ω) interact strongly with nucleons and
they decay quickly to Λ (reactions with strangeness conversation) → hypernucleus is not produced. First discoveries (1952) during cosmic rays studies. Today more than 33 hypernuclei are known. Production by intensive meson beams. Decay time τ ≈ τΛ ≈10-10s.
They make possible to study influence of strangeness on nuclear force properties – demonstrate existence of attractive forces between Λ and nucleons (BΛp < Bnp).
Antinuclei: antiproton, antineutron, antilambda, pozitron and other antiparticles are produced.
Possible existence of antinuclei. Up to now only the lights: antideuteron, antihelium 3
Antiatoms: First antiatom (antihydrogen) at CERN (1996) – creation of electron and positron pair during antiproton movement through electromagnetic field of nuclei was used (it resolves problem of positron capture by antiproton).
One case of antihydrogen anihilation –
production of 4 mesons (p + anti-p)
and 2 (e + e+)
Antiproton decelerator at CERN makes possible production of
thousands antihydrogens, capture of antiprotons to
magnetic trap, mixture with positrons → creation of
antihydrogen – detection by anihilation
Exotic atoms: 1) mion atoms – electron is changed by mion
2) positronium – bound system consists of electron
3) antiprotonic helium atoms – bound system consists
of nucleus and antiproton
Halo nuclei: consist of strongly bounded core
often stable isotope and very weak bounded
neutrons or protons around
Borromean nuclei: weakly bound system, every
its part is not bounded alone
Nature of nuclear forces
The forces inside nuclei are electromagnetic interaction (Coulomb repulsion), weak (beta decay)
but mainly strong nuclear interaction (it bonds nucleus together).
For Coulomb interaction binding energy is B Z (Z-1)B/Z Z for large Z non saturated
forces with long range.
For nuclear force binding energy is B/A const – done byshort range and saturation
of nuclear forces.Maximal range ~1.7 fm
Nuclear forces are attractive (bond nucleus together), for very short distances (~0.4 fm) they
are repulsive (nucleus does not collapse). More accurate form of nuclear force potential can be obtained by scattering of nucleons on nucleons or nuclei.
Charge independency – cross sections of nucleon scattering are not dependent on their electric charge. → For nuclear forces neutron and proton are two different states of single particle - nucleon. New quantity isospin T is define for their description. Nucleon has than isospin T = 1/2 with two possible orientation TZ = +1/2 (proton) and TZ = -1/2 (neutron). Formally we work with isospin as with spin.
Spin dependence – explains existence of stable deuteron (it exists only at triplet state – s = 1 and no at singlet - s = 0) and absence of di-neutron. This property is studied by scattering experiments using oriented beams and targets.
Tenzor charakter – interaction between two nucleons depends on angle between spin directions and directionof join of particles.
Expect strong interaction electric force influences also. Nucleus has positive charge and for positive charged particle this force produces Coulomb barrier (range of electric force is larger then this of strong force). Appropriate potential has form V(r) ~ Q/r.
In the case of scattering centrifugal barier given by angular momentum of incident particle acts in addition.
Exchange nature of nuclear forces:
short range → nonzero rest mass of intermediate particles. H. Yukawa proposed corresponding potential
where m is mass of intermediate particle and ћ /mc is its Compton wave length. We put Compton length equal to range R of nuclear forces and we determine mass of intermediate particle:
Intermediate particles with similar masses were discovered and named as π mesons. Attractive
and repulsive nuclear force is than intermediated exchange of charged and neutral mesons:
p + π - → n, n + π + → p, p + π0 → p, n + π0 → n
Protons and neutrons emit and absorb mesons. Why their masses are not changed?
Uncertainty principle: ΔEΔt ≥ ћ → violation of energy conservation is allowed if it is shorter then ћ/ΔE. Maximal range of nuclear forces is R = 1.7 fm. Then the smallest time of nucleon transit is: Δt = R/c. Value of violation of energy conservation is during emission of meson with mass mπ: ΔE = mπc2. If time of violation will be Δt we obtain for maximal possible energy violation (meson mass): mπc2 = ћc/R (the same as earlier shown)
Further mesons (η, ρ, φ …) were found, also two-meson exchange.